Tetrahedron p. 11445 - 11462 (1996)
Update date:2022-08-05
Topics:
Bowman, W. Russell
Stephenson, Peter T.
Young, Adrian R.
Cascade radical reactions, initiated by cyclisation of sp3 carbon-centred radicals onto the C-atom of imines, have been used to develop a new protocol for the synthesis of a range of nitrogen heterocycles. The C-centred radical intermediates were generated from benzeneselenyl precursors using Bu3SnH. The aminyl radicals generated by cyclisation onto imines undergo further 5- or 6-exo cyclisation with suitably placed alkenes.
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