1172ꢀ
JieꢀLiꢀetꢀal.ꢀ/ꢀChineseꢀJournalꢀofꢀCatalysisꢀ38ꢀ(2017)ꢀ1166–1173ꢀ
Cong,ꢀW.ꢀX.ꢀZhang,ꢀJ.ꢀH.ꢀLuo,ꢀS.ꢀLi,ꢀZ.ꢀL.ꢀWang,ꢀJ.ꢀChem.ꢀSci.,ꢀ2014,ꢀ
26,ꢀ141–145.ꢀ
7] Y.ꢀ Hara,ꢀ H.ꢀ Kusaka,ꢀ H.ꢀ Inagaki,ꢀ K.ꢀ Takahashi,ꢀ K.ꢀ Wada,ꢀ J.ꢀ Catal.,ꢀ
000,ꢀ194,ꢀ188–197.ꢀ
8] Y.ꢀQ.ꢀ Huang,ꢀ Y.ꢀ Ma,ꢀY.ꢀW.ꢀ Cheng,ꢀ L.ꢀJ.ꢀ Wang,ꢀ X.ꢀ Li,ꢀ Appl.ꢀCatal.ꢀA,ꢀ
015,ꢀ495,ꢀ124–130.ꢀ
1
[
[
2
2
(
(
2)
1)
[9] G.ꢀBudroni,ꢀA.ꢀCorma,ꢀJ.ꢀCatal.,ꢀ2008,ꢀ257,ꢀ403–408.ꢀ
10] J.ꢀ Li,ꢀ W.ꢀ P.ꢀ Tian,ꢀ L.ꢀ Shi,ꢀ Ind.ꢀ Eng.ꢀ Chem.ꢀ Res.,ꢀ 2010,ꢀ 49,ꢀ
[
[
[
[
[
[
11837–11840.ꢀ
11] Y.ꢀYu,ꢀY.ꢀL.ꢀGuo,ꢀW.ꢀC.ꢀZhan,ꢀY.ꢀGuo,ꢀY.ꢀS.ꢀWang,ꢀG.ꢀZ.ꢀLu,ꢀJ.ꢀMol.ꢀCatal.ꢀ
A,ꢀ2014,ꢀ392,ꢀ1–7.ꢀ
12] Y.ꢀYu,ꢀW.ꢀC.ꢀZhan,ꢀY.ꢀGuo,ꢀG.ꢀZ.ꢀLu,ꢀS.ꢀAdjimi,ꢀY.ꢀL.ꢀGuo,ꢀJ.ꢀMol.ꢀCatal.ꢀA,ꢀ
2014,ꢀ395,ꢀ392–397.ꢀ
13] C.ꢀI.ꢀMeyer,ꢀS.ꢀA.ꢀRegenhardt,ꢀA.ꢀJ.ꢀMarchi,ꢀT.ꢀF.ꢀGaretto,ꢀAppl.ꢀCatal.ꢀ
A,ꢀ2012,ꢀ417–418,ꢀ59–65.ꢀ
14] S.ꢀA.ꢀRegenhardt,ꢀC.ꢀI.ꢀMeyer,ꢀT.ꢀF.ꢀGaretto,ꢀA.ꢀJ.ꢀMarchi,ꢀAppl.ꢀCatal.ꢀ
A,ꢀ2012,ꢀ449,ꢀ81–87.ꢀ
1
00
50
0
-50
15] W.ꢀT.ꢀHuo,ꢀC.ꢀL.ꢀZhang,ꢀH.ꢀJ.ꢀYuan,ꢀM.ꢀJ.ꢀJia,ꢀC.ꢀL.ꢀNing,ꢀY.ꢀTang,ꢀY.ꢀ
Zhang,ꢀJ.ꢀH.ꢀLuo,ꢀZ.ꢀL.ꢀWang,ꢀW.ꢀX.ꢀZhang,ꢀJ.ꢀInd.ꢀEng.ꢀChem.,ꢀ2014,ꢀ
Fig.ꢀ 15.ꢀ 27Alꢀ MASꢀ NMRꢀ spectraꢀ ofꢀ theꢀ freshꢀ (1)ꢀ andꢀ usedꢀ (2)
20,ꢀ4140–4145.ꢀ
Ni(5%)/Al
2
3
O .ꢀ
[
16] Y.ꢀZhang,ꢀL.ꢀL.ꢀZhao,ꢀH.ꢀX.ꢀZhang,ꢀH.ꢀT.ꢀLi,ꢀP.ꢀP.ꢀLiu,ꢀY.ꢀY.ꢀGai,ꢀY.ꢀX.ꢀ
Zhao,ꢀCIESC.,ꢀ2015,ꢀ66,ꢀ2505–2513.ꢀ
[17] C.ꢀ I.ꢀ Meyer,ꢀ S.ꢀ A.ꢀ Regenhardt,ꢀ M.ꢀ E.ꢀ Bertone,ꢀ A.ꢀ J.ꢀ Marchi,ꢀ T.ꢀ F.ꢀ
Garetto,ꢀCatal.ꢀLett.,ꢀ2013,ꢀ143,ꢀ1067–1073.ꢀ
[
[
[
[
18] J.ꢀLi,ꢀW.ꢀP.ꢀTian,ꢀX.ꢀWang,ꢀL.ꢀShi,ꢀChem.ꢀEng.ꢀJ.,ꢀ2011,ꢀ175,ꢀ417–422.ꢀ
19] W.ꢀP.ꢀTian,ꢀS.ꢀF.ꢀGuo,ꢀL.ꢀShi,ꢀPet.ꢀSci.ꢀTechnol.,ꢀ2014,ꢀ32,ꢀ1784–1790.ꢀ
20] S.ꢀF.ꢀGuo,ꢀL.ꢀShi,ꢀCatal.ꢀToday,ꢀ2013,ꢀ212,ꢀ137–141.ꢀ
21] M.ꢀ E.ꢀ Bertone,ꢀ S.ꢀ A.ꢀ Regenhardt,ꢀ C.ꢀ I.ꢀ Meyer,ꢀ V.ꢀ Sebastian,ꢀ T.ꢀ F.ꢀ
Garetto,ꢀA.ꢀJ.ꢀMarchi,ꢀTop.ꢀCatal.,ꢀ2016,ꢀ59,ꢀ159–167.ꢀ
(
2)
1)
[22] P.ꢀG.ꢀSavva,ꢀK.ꢀGoundani,ꢀJ.ꢀVakros,ꢀK.ꢀBourikas,ꢀC.ꢀFountzoula,ꢀD.ꢀ
Vattis,ꢀ A.ꢀ Lycourghiotis,ꢀ C.ꢀ Kordulis,ꢀ Appl.ꢀ Catal.ꢀ B,ꢀ 2008,ꢀ 79,ꢀ
(
1
99–207.ꢀ
23] A.ꢀL.ꢀAlberton,ꢀM.ꢀM.ꢀV.ꢀMꢀSouza,ꢀM.ꢀSchmal,ꢀCatal.ꢀToday,ꢀ2007,ꢀ
23,ꢀ257–264.ꢀ
[
1
[
24] B.ꢀC.ꢀLippens,ꢀJ.ꢀH.ꢀdeꢀBoer,ꢀActaꢀCrystal,ꢀ1964,ꢀ17,ꢀ1312–1321.ꢀ
25] H.ꢀ T.ꢀ Li,ꢀ Y.ꢀ L.ꢀ Xu,ꢀ C.ꢀ G.ꢀ Gao,ꢀ Y.ꢀ X.ꢀ Zhao,ꢀ Catal.ꢀ Today,ꢀ 2010,ꢀ
4.ꢀ ꢀ Conclusionsꢀ
[
158,475–480.ꢀ
2 3
AꢀseriesꢀofꢀNi/Al O ꢀspinel‐derivedꢀcatalystsꢀwithꢀdifferentꢀ
[26] G.ꢀPaglia,ꢀC.ꢀE.ꢀBuckley,ꢀA.ꢀL.ꢀRohl,ꢀR.ꢀD.ꢀHart,ꢀK.ꢀWinter,ꢀA.ꢀJ.ꢀStuder,ꢀ
levelsꢀofꢀNi‐loadingꢀ(2.5,ꢀ5ꢀandꢀ7.5)ꢀwt%ꢀwereꢀsynthesizedꢀandꢀ
studiedꢀforꢀtheꢀlow‐temperatureꢀhydrogenationꢀofꢀMAꢀtoꢀpro‐
duceꢀ SA.ꢀ Optimizedꢀ preparationꢀ conditionsꢀ (5%ꢀ Ni‐loading,ꢀ
reductionꢀatꢀ700ꢀ°Cꢀforꢀ2ꢀh)ꢀyieldedꢀaꢀcatalystꢀthatꢀpossessedꢀaꢀ
largeꢀ amountꢀ ofꢀ well‐dispersed,ꢀ smallꢀ Ni ꢀ particlesꢀ yieldingꢀ
highꢀcatalyticꢀactivityꢀunderꢀoptimizedꢀreactionꢀconditionsꢀ(120ꢀ
B.ꢀA.ꢀHunter,ꢀJ.ꢀV.ꢀHanna,ꢀChem.ꢀMater.,ꢀ2004,ꢀ16,ꢀ220–236.ꢀ
27] Z.ꢀG.ꢀHao,ꢀQ.ꢀS.ꢀZhu,ꢀZ.ꢀJiang,ꢀB.ꢀL.ꢀHou,ꢀH.ꢀZ.ꢀLi,ꢀFuelꢀProcess.ꢀTechnol.,ꢀ
[
2009,ꢀ90,ꢀ113–121.ꢀ
[
28] G.ꢀH.ꢀLi,ꢀL.ꢀJ.ꢀHu,ꢀJ.ꢀM.ꢀHill,ꢀAppl.ꢀCatal.ꢀA,ꢀ2006,ꢀ301,ꢀ16–24.ꢀ
29] Z.ꢀMa,ꢀQ.ꢀZ.ꢀJiang,ꢀX.ꢀWang,ꢀW.ꢀG.ꢀZhang,ꢀZ.ꢀF.ꢀMa,ꢀCatal.ꢀCommun.,ꢀ
[
0
2
012,ꢀ17,ꢀ49–53.ꢀ
30] G.ꢀ Poncelet,ꢀ M.ꢀ A.ꢀ Centeno,ꢀ R.ꢀ Molina,ꢀ Appl.ꢀ Catal.ꢀ A,ꢀ 2005,ꢀ 288,ꢀ
32–242.ꢀ
[
[
°
Cꢀandꢀ0.5ꢀMPaꢀofꢀH
achieved,ꢀ withꢀ aꢀ constantꢀ near‐100%ꢀ conversionꢀ ofꢀ MAꢀ andꢀ
90%ꢀselectivityꢀtoꢀSA.ꢀ
2
).ꢀLong‐termꢀ stabilityꢀ forꢀoverꢀ 72ꢀ hꢀwasꢀ
2
31] Z.ꢀBoukha,ꢀC.ꢀJimenez‐Gonzalez,ꢀB.ꢀdeꢀRivas,ꢀJ.ꢀR.ꢀGonzalez‐Velasco,ꢀ
~
J.ꢀ I.ꢀ Gutierrez‐Ortiz,ꢀ R.ꢀ Lopez‐Fonseca,ꢀ Appl.ꢀ Catal.ꢀ B,ꢀ 2014,ꢀ
158–159,ꢀ190–201.ꢀ
Referencesꢀ
[32] R.ꢀ Lopez‐Fonseca,ꢀ C.ꢀ Jimenez‐Gonzalez,ꢀ B.ꢀ deꢀ Rivas,ꢀ J.I.ꢀ
Gutierrez‐Ortiz,ꢀAppl.ꢀCatal.ꢀA,ꢀ2012,ꢀ437–438,ꢀ53–62.ꢀ
[
[
[
[
[
[
33] F.ꢀMeyer,ꢀR.ꢀHempelmann,ꢀS.ꢀMathurband,ꢀM.ꢀVeith,ꢀJ.ꢀMater.ꢀChem.,ꢀ
999,ꢀ9,ꢀ1755–1763.ꢀ
34] C.ꢀRagupathi,ꢀJ.ꢀJ.ꢀVijaya,ꢀP.ꢀSurendhar,ꢀL.ꢀJ.ꢀKennedy,ꢀPolyhedron,ꢀ
014,ꢀ72,1–7.ꢀ
35] R.ꢀWang,ꢀY.ꢀH.ꢀLi,ꢀR.ꢀH.ꢀShi,ꢀM.ꢀM.ꢀYang,ꢀJ.ꢀMol.ꢀCatal.ꢀA,ꢀ2011,ꢀ344,ꢀ
22–127.ꢀ
36] T.ꢀNumaguchi,ꢀ H.ꢀ Eida,ꢀK.ꢀShoji,ꢀ Int.ꢀJ.ꢀHydrog.ꢀEnergy,ꢀ1997,ꢀ22,ꢀ
111–1115.ꢀ
37] M.ꢀ Tao,ꢀ X.ꢀ Meng,ꢀ Y.ꢀ H.ꢀ Lu,ꢀ Z.ꢀ C.ꢀ Bian,ꢀ Z.ꢀ Xin,ꢀ Fuel,ꢀ 2016,ꢀ 165,ꢀ
89–297.ꢀ
38] Y.ꢀH.ꢀFeng,ꢀH.ꢀB.ꢀYin,ꢀA.ꢀL.ꢀWang,ꢀT.ꢀXie,ꢀT.ꢀS.ꢀJiang,ꢀAppl.ꢀCatal.ꢀA,ꢀ
[
[
[
[
[
[
1] C.ꢀI.ꢀMeyer,ꢀA.ꢀJ.ꢀMarchi,ꢀA.ꢀMonzon,ꢀT.ꢀF.ꢀGaretto,ꢀAppl.ꢀCatal.ꢀA,ꢀ
1
2009,ꢀ367,ꢀ122–129.ꢀ
2] R.ꢀC.ꢀZhang,ꢀH.ꢀB.ꢀYin,ꢀD.ꢀZ.ꢀZhang,ꢀL.ꢀQi,ꢀH.ꢀH.ꢀLu,ꢀY.ꢀT.ꢀShen,ꢀT.ꢀS.ꢀ
Jiang,ꢀChem.ꢀEng.ꢀJ.,ꢀ2008,ꢀ140,ꢀ488–496.ꢀ
3] D.ꢀZ.ꢀGao,ꢀY.ꢀH.ꢀFeng,ꢀH.ꢀB.ꢀYin,ꢀA.ꢀL.ꢀWang,ꢀT.ꢀS.ꢀJiang,ꢀChem.ꢀEng.ꢀJ.,ꢀ
2
1
2
013,ꢀ233,ꢀ349–359.ꢀ
4] X.ꢀLiao,ꢀY.ꢀZhang,ꢀM.ꢀHill,ꢀX.ꢀXia,ꢀY.ꢀX.ꢀZhao,ꢀZ.ꢀJiang,ꢀAppl.ꢀCatal.ꢀA,ꢀ
014,ꢀ488,ꢀ256–264.ꢀ
5] J.ꢀLi,ꢀL.ꢀP.ꢀQian,ꢀL.ꢀY.ꢀHu,ꢀB.ꢀYue,ꢀH.ꢀY.ꢀHe,ꢀChin.ꢀChem.ꢀLett.,ꢀ2016,ꢀ27,ꢀ
004–1008.ꢀ
6] H.ꢀJ.ꢀYuan,ꢀC.ꢀL.ꢀZhang,ꢀW.ꢀT.ꢀHuo,ꢀC.ꢀL.ꢀNing,ꢀY.ꢀTang,ꢀY.ꢀZhang,ꢀD.ꢀQ.ꢀ
1
2
2
1