Tetrahedron p. 7417 - 7428 (1997)
Update date:2022-08-30
Topics:
Barton, Derek H.R.
Costas Salgueiro, Miquel
MacKinnon, John
The functionalization of saturated hydrocarbons utilizing the Gif oxidation system is considered to occur via an intermediate containing an Fe-C bond. Iodine and iodide ion have been found to capture efficiently the Fe-C bond to give the corresponding alkyl iodide in both the Fe(II)-Fe(IV) and Fe(III)-Fe(V) manifolds. This trapping of the Fe-C bond in both manifolds is shown to be non-radical in nature.
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