Tetrahedron p. 3473 - 3486 (1996)
Update date:2022-08-16
Topics:
Heaney, Harry
Papageorgiou, George
A series of bis(aminol) ethers were prepared from primary aliphatic amines and benzylamine together with formaldehyde and either ethanol or methanol; they were reacted with electrophiles to give N-alkyl-N-alkoxymethyl-methyleneiminium salts which gave mixtures of secondary and tertiary amines in reactions with electron rich aromatic compounds: sequential reactions with two different nucleophiles gave the expected tertiary amines.
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