Chemistry Letters p. 565 - 568 (1983)
Update date:2022-08-29
Topics:
Okamoto, Yasuaki
Matsunaga, Etsuo
Imanaka, Toshinobu
Teranishi, Shiichiro
It was found with CO/H2 reaction over unsupported Ni catalysts that the C2+/CH4 selectivity decreased in the order; Ni-boride > Raney-Ni > Decomposed-Ni ca.Ni-phosphide.This suggests that both the activity and selectivity increase as the electron density on Ni metal increases.The H/C atomic ratio of the surface carbon species deposited during the reaction was also dependent on the catalyst.
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