Bulletin of the Chemical Society of Japan p. 2898 - 2901 (1982)
Update date:2022-08-12
Topics:
Murakami, Yukito
Aoyama, Yasuhiro
Kikuchi, Jun-ichi
As regards the effect of zinc(II) ion on the reduction of hexachloroacetone, the kinetic activity of a <20>paracyclophane (PCP) bearing 1,4-dihydronicotinamide (HNA) and 2-pyridinecarboxylic acid (Py) moieties, HNA-PCP-Py, has been investigated as an alcohol dehydrogenase model in reference to that of PCP-HNA in the light of their metal-coordination behavior.The reduction ability of PCP-HNA was significantly lowered as it underwent complex formation with zinc.On the other hand, HNA-PCP-Py showed an apparent rate maximum in a relatively lower concentration range of ZnCl2.The kinetic behavior was analyzed on the basis of the formation of two kinds of zinc complexes of HNA-PCP-Py: the 1:1 complex
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