Tetrahedron Letters p. 6499 - 6502 (1999)
Update date:2022-08-16
Topics:
Montana, Angel M.
Fernandez, David
An enantioselective synthetic methodology to prepare trans-fused bicyclo[5.3.0]decane systems is presented. It is a very versatile methodology based on two key reactions: [4+3] cycloaddition reaction (to generate the seven-membered ring) and the Nicholas reaction (that facilitates the insertion of the five-membered ring). This methodology allows the easy preparation of a wide range of bioactive natural products containing the transfused bicyclo[5.3.0]decane system. The application of this methodology to the enantioselective synthetic approach to the pseudoguaiane carbon- skeleton is described.
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