Journal of Chemical Physics p. 9081 - 9085 (1992)
Update date:2022-08-31
Topics:
Hassoon, S.
Snavely, D. L.
Oref, I.
The two-photon photodissociation of gaseous azulene at 325 nm is reported.Acetylene is the major photodissociation product.The quantum yields for acetylene produced by irradiation of neat azulene at its normal vapor pressure and as a function of argon bath gas pressure are reported.The quantum yield of acetylene produced from irradiated azulene at its normal vapor pressure (ca. 10 m Torr) is ca. (5.85+/-1.46) * 10-6.Using a mechanism by which internal conversion precedes the absorption of the second photon, the two-photon absorption cross section is calculated.
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