Tetrahedron Letters p. 4165 - 4168 (1992)
Update date:2022-07-31
Topics:
Tanaka
Mukaiyama
Mitsuhashi
Wakamatsu
The total synthesis of gomisin A and schizandrin having natural configurations were accomplished for the first time. The key feature of these syntheses is a highly efficient intramolecular oxidative coupling of the intermediates 9 and 21, which can be obtained as both enantiomers in optically pure forms. The manipulation of the lactone moieties of 7 and 22 afforded natural enantiomers of schizandrin and gomisin A.
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Doi:10.1016/S0040-4020(01)80521-4
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(1992)